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Development of combined coagulation-hydrolysis acidification-dynamic membrane bioreactor system for treatment

Xue Shen, Lei Lu, Baoyu Gao, Xing Xu, Qinyan Yue

《环境科学与工程前沿（英文）》 2019年 第13卷 第1期 doi: 10.1007/s11783-019-1093-8

摘要：

• We created a combined system for treating oilfield polymer-flooding wastewater.

• The system was composed of coagulation, hydrolysis acidification and DMBR.

• Coagulant integrated with demulsifier dominated the removal of crude oil.

• The DMBR proceed efficiently without serious membrane fouling.

关键词： Coagulation     Hydrolysis acidification     Dynamic membrane bioreactor     Polymer flooding    

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Methanation and chemolitrophic nitrogen removal by an anaerobic membrane bioreactor coupled partial nitrification

《环境科学与工程前沿（英文）》 2023年 第17卷 第6期 doi: 10.1007/s11783-023-1668-2

摘要：

● Efficient carbon methanation and nitrogen removal was achieved in AnMBR-PN/A system.

关键词： Anaerobic membrane bioreactor     Partial nitrification/Anammox     Carbon separation     Chemolitrophic nitrogen removal    

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Recent advances in membrane bioreactor technology for wastewater treatment in China

Xia HUANG, Kang XIAO, Yuexiao SHEN

《环境科学与工程前沿（英文）》 2010年 第4卷 第3期   页码 245-271 doi: 10.1007/s11783-010-0240-z

摘要： Since the introduction of the membrane bioreactor (MBR) in China in the early 1990s, remarkable progress has been achieved on the research and application of this technology. China has now become one of the most active fields in the world in this regard. This review outlines the development of MBR-based processes in China and their performance of treating municipal and industrial wastewaters. Since membrane fouling is a critical operational problem with MBR processes, this paper also proposes updated understanding of fouling mechanisms and strategies of fouling control, which are mainly compiled from publications of Chinese researchers. As for the commercial application of MBR in the country, the latest statistics of large-scale MBR plants (>10000 m·d) are provided, and the growth trend of total treatment capacity as well as its driving force is analyzed.

关键词： membrane bioreactor (MBR)     municipal wastewater treatment     industrial wastewater treatment     membrane fouling     commercial application     China    

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Bisphenol A removal from synthetic municipal wastewater by a bioreactor coupled with either a forwardosmotic membrane or a microfiltration membrane unit

Hongtao ZHU, Wenna LI

《环境科学与工程前沿（英文）》 2013年 第7卷 第2期   页码 294-300 doi: 10.1007/s11783-013-0486-3

摘要： Forward osmotic membrane bioreactor is an emerging technology that combines the advantages of forward osmosis and conventional membrane bioreactor. In this paper, bisphenol A removal by using a forward osmotic membrane bioreactor and a conventional membrane bioreactor that shared one biologic reactor was studied. The total removal rate of bisphenol A by the conventional membrane bioreactor and forward osmotic membrane bioreactor was as high as 93.9% and 98%, respectively. Biodegradation plays a dominant role in the total removal of bisphenol A in both processes. In comparison of membrane rejection, the forward osmosis membrane can remove approximately 70% bisphenol A from the feed, much higher than that of the microfiltration membrane (below 10%). Forward osmosis membrane bioreactor should be operated with its BPA loading rate under 0.08 mg·g ·d to guarantee the effluent bisphenol A concentration less than10 μg·L .

关键词： forward osmosis     membrane bioreactor     bisphenol A     microfiltration    

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Enhanced atrazine removal using membrane bioreactor bioaugmented with genetically engineered microorganism

LIU Chun, HUANG Xia

《环境科学与工程前沿（英文）》 2008年 第2卷 第4期   页码 452-460 doi: 10.1007/s11783-008-0050-8

摘要： Bioaugmentation with genetically engineered microorganisms (GEMs) in a membrane bioreactor (MBR) for enhanced removal of recalcitrant pollutants was explored. An atrazine-degrading genetically engineered microorganism (GEM) with green fluorescent protein was inoculated into an MBR and the effects of such a bioaugmentation strategy on atrazine removal were investigated. The results show that atrazine removal was improved greatly in the bioaugmented MBR compared with a control system. After a start-up period of 6 days, average 94.7% of atrazine was removed in bioaugmented MBR when atrazine concentration of influent was 14.5 mg/L. The volumetric removal rates increased linearly followed by atrazine loading increase and the maximum was 65.5 mg/(L·d). No negative effects were found on COD removal although carbon oxidation activity of bioaugmented sludge was lower than that of common sludge. After inoculation, adsorption to sludge flocs was favorable for GEM survival. The GEM population size initially decreased shortly and then was kept constant at about 10–10 CFU/mL. Predation of micro-organisms played an important role in the decay of the GEM population. GEM leakage from MBR was less than 10 CFU/mL initially and was then undetectable. In contrast, in a conventionally activated sludge bioreactor (CAS), sludge bulking occurred possibly due to atrazine exposure, resulting in bioaugmentation failure and serious GEM leakage. So MBR was superior to CAS in atrazine bioaugmentation treatment using GEM.
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characteristics of wastewater treatment plants retrofitted from the conventional activated sludge process to the membranebioreactor process

《环境科学与工程前沿（英文）》 doi: 10.1007/s11783-021-1483-6

摘要：

While a growing number of wastewater treatment plants (WWTPs) are being retrofitted from the conventional activated sludge (CAS) process to the membrane bioreactor (MBR) process, the debate on the techno-economy of MBR vs. CAS has continued and calls for a thorough assessment based on techno-economic valuation.

关键词： Membrane bioreactor (MBR)     Conventional activated sludge (CAS)     Cost-benefit analysis     Data envelopment analysis     Net profit    

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Energy reduction of a submerged membrane bioreactor using a polytetrafluoroethylene (PTFE) hollow-fibermembrane

Taro Miyoshi, Thanh Phong Nguyen, Terumi Tsumuraya, Hiromu Tanaka, Toru Morita, Hiroki Itokawa, Toshikazu Hashimoto

《环境科学与工程前沿（英文）》 2018年 第12卷 第3期 doi: 10.1007/s11783-018-1018-y

摘要： In this study, we modified a polytetrafluoroethylene (PTFE) hollow-fiber membrane element used for submerged membrane bioreactors (MBRs) to reduce the energy consumption during MBR processes. The high mechanical strength of the PTFE membrane made it possible to increase the effective length of the membrane fiber from 2 to 3 m. In addition, the packing density was increased by 20% by optimizing the membrane element configuration. These modifications improve the efficiency of membrane cleaning associated with aeration. The target of specific energy consumption was less than 0.4 kWh·m in this study. The continuous operation of a pilot MBR treating real municipal wastewater revealed that the MBR utilizing the modified membrane element can be stably operated under a specific air demand per membrane surface area (SAD ) of 0.13 m ·m ·hr when the daily-averaged membrane fluxes for the constant flow rate and flow rate fluctuating modes of operation were set to 0.6 and 0.5 m ·m ·d , respectively. The specific energy consumption under these operating conditions was estimated to be less than 0.37 kWh·m . These results strongly suggest that operating an MBR equipped with the modified membrane element with a specific energy consumption of less than 0.4 kWh·m is highly possible.

关键词： Energy-saving     Membrane bioreactor     Polytetrafluoroethylene (PTFE) membrane     Hollow fiber     Power consumption    

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Performance of bioferric-submerged membrane bioreactor for dyeing wastewater treatment

ZOU Haiyan, XI Danli

《环境科学与工程前沿（英文）》 2007年 第1卷 第3期   页码 374-380 doi: 10.1007/s11783-007-0064-7

摘要： Adding iron salt or iron hydroxide to sludgemixed liquor in an aeration tank of a conventional activated sludge processes (bioferric process) can simultaneously improve the sludge s filterability and enhance the system s treatment capacity. In view of this, Fe(OH) was added to a submerged membrane bioreactor (SMBR) to enhance the removal efficiency and to mitigate membrane fouling. Bioferric process and SMBR were combined to create a novel process called Bioferric-SMBR. A side-by-side comparison study of Bioferric-SMBR and common SMBR dealing with dyeing wastewater was carried out. Bioferric-SMBR showed potential superiority, which could enhance removal efficiency, reduce membrane fouling and improve sludge characteristic. When volumetric loading rate was 25% higher than that of common SMBR, the removal efficiencies of Bioferric-SMBR on COD, dye, and NH-N were 1.0%, 9.5%, and 5.2% higher than that of common SMBR, respectively. The trans-membrane pressure of Bioferric-SMBR was only 36% of that in common SMBR while its membrane flux was 25% higher than that of common SMBR. The stable running period in Bioferric-SMBR was 2.5 times of that in common SMBR when there was no surplus sludge discharged. The mixed liquor suspended solids concentration of Bioferric-SMBR was higher than that of common SMBR with more diversified kinds of microorganisms such as protozoans and metazoans. The mean particle diameter and specific oxygen uptake rate of Bioferric-SMBR were 3.10 and 1.23 times the common SMBR, respectively.

关键词： hydroxide     surplus     aeration     SMBR     Bioferric process    

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Membrane bioreactors for hospital wastewater treatment: recent advancements in membranes and processes

《化学科学与工程前沿（英文）》 2022年 第16卷 第5期   页码 634-660 doi: 10.1007/s11705-021-2107-1

摘要： Discharged hospital wastewater contains various pathogenic microorganisms, antibiotic groups, toxic organic compounds, radioactive elements, and ionic pollutants. These contaminants harm the environment and human health causing the spread of disease. Thus, effective treatment of hospital wastewater is an urgent task for sustainable development. Membranes, with controllable porous and nonporous structures, have been rapidly developed for molecular separations. In particular, membrane bioreactor (MBR) technology demonstrated high removal efficiency toward organic compounds and low waste sludge production. To further enhance the separation efficiency and achieve material recovery from hospital waste streams, novel concepts of MBRs and their applications are rapidly evolved through hybridizing novel membranes (non hydrophilic ultrafiltration/microfiltration) into the MBR units (hybrid MBRs) or the MBR as a pretreatment step and integrating other membrane processes as subsequent secondary purification step (integrated MBR-membrane systems). However, there is a lack of reviews on the latest advancement in MBR technologies for hospital wastewater treatment, and analysis on its major challenges and future trends. This review started with an overview of main pollutants in common hospital wastewater, followed by an understanding on the key performance indicators/criteria in MBR membranes (i.e., solute selectivity) and processes (e.g., fouling). Then, an in-depth analysis was provided into the recent development of hybrid MBR and integrated MBR-membrane system concepts, and applications correlated with wastewater sources, with a particular focus on hospital wastewaters. It is anticipated that this review will shed light on the knowledge gaps in the field, highlighting the potential contribution of hybrid MBRs and integrated MBR-membrane systems toward global epidemic prevention.

关键词： membrane technology     membrane bioreactor     hospital wastewater     hybrid MBR     integrated MBR-membrane system    

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Engineering application of membrane bioreactor for wastewater treatment in China: Current state and future

Kang XIAO, Ying XU, Shuai LIANG, Ting LEI, Jianyu SUN, Xianghua WEN, Hongxun ZHANG, Chunsheng CHEN, Xia HUANG

《环境科学与工程前沿（英文）》 2014年 第8卷 第6期   页码 805-819 doi: 10.1007/s11783-014-0756-8

摘要： China has been the forerunner of large-scale membrane bioreactor (MBR) application. Since the first large-scale MBR (≥10 000 m ·d ) was put into operation in 2006, the engineering implementation of MBR in China has attained tremendous development. This paper outlines the commercial application of MBR since 2006 and provides a variety of engineering statistical data, covering the fields of municipal wastewater, industrial wastewater, and polluted surface water treatment. The total treatment capacity of MBRs reached 1 × 10 m ·d in 2010, and has currently exceeded 4.5 × 10 m ·d with ~75% of which pertaining to municipal wastewater treatment. The anaerobic/anoxic/aerobic-MBR and its derivative processes have been the most popular in the large-scale municipal application, with the process features and typical ranges of parameters also presented in this paper. For the treatment of various types of industrial wastewater, the configurations of the MBR-based processes are delineated with representative engineering cases. In view of the significance of the cost issue, statistics of capital and operating costs are also provided, including cost structure and energy composition. With continuous stimulation from the environmental stress, political propulsion, and market demand in China, the total treatment capacity is expected to reach 7.5 × 10 m ·d by 2015 and a further expansion of the market is foreseeable in the next five years. However, MBR application is facing several challenges, such as the relatively high energy consumption. Judging MBR features and seeking suitable application areas should be of importance for the long-term development of this technology.

关键词： membrane bioreactor (MBR)     engineering application     wastewater treatment     review     China    

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Effects of hydraulic retention time on net present value and performance in a membrane bioreactor treating

Dawei Yu, Jianxing Wang, Libin Zheng, Qianwen Sui, Hui Zhong, Meixue Cheng, Yuansong Wei

《环境科学与工程前沿（英文）》 2020年 第14卷 第6期 doi: 10.1007/s11783-020-1280-7

摘要： Abstract • The membrane bioreactor cost decreased by 38.2% by decreasing HRT from 72 h to 36 h. • Capital and operation costs contributed 62.1% and 37.9% to decreased costs. • The membrane bioreactor is 32.6% cheaper than the oxidation ditch for treatment. • The effluent COD also improved from 709.93±62.75 mg/L to 280±17.32 mg/L. • Further treatment also benefited from lower pretreatment investment. A cost sensitivity analysis was performed for an industrial membrane bioreactor to quantify the effects of hydraulic retention times and related operational parameters on cost. Different hydraulic retention times (72–24 h) were subjected to a flat-sheet membrane bioreactor updated from an existing 72 h oxidation ditch treating antibiotic production wastewater. Field experimental data from the membrane bioreactor, both full-scale (500 m3/d) and pilot (1.0 m3/d), were used to calculate the net present value (NPV), incorporating both capital expenditure (CAPEX) and operating expenditure. The results showed that the tank cost was estimated above membrane cost in the membrane bioreactor. The decreased hydraulic retention time from 72 to 36 h reduced the NPV by 38.2%, where capital expenditure contributed 24.2% more than operational expenditure. Tank construction cost was decisive in determining the net present value contributed 62.1% to the capital expenditure. The membrane bioreactor has the advantage of a longer lifespan flat-sheet membrane, while flux decline was tolerable. The antibiotics decreased to 1.87±0.33 mg/L in the MBR effluent. The upgrade to the membrane bioreactor also benefited further treatments by 10.1%–44.7% lower direct investment.

关键词： Antibiotic production wastewater     Net present value     Membrane bioreactor     Hydraulic retention time     Pollutant removal    

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Relationship between sludge settleability and membrane fouling in a membrane bioreactor

SUN Yujiao, WANG Yong, HUANG Xia

《环境科学与工程前沿（英文）》 2007年 第1卷 第2期   页码 221-225 doi: 10.1007/s11783-007-0038-9

摘要： The evolution of activated sludge settleability and its relationship to membrane fouling in a submerged membrane bioreactor were studied at a lab-scale equipment fed with synthetic wastewater. It was found that sludge volume index (SVI) gradually increased and the sludge settleability was reduced, which was caused by the propagation of filamentous bacteria. With increasing SVI, the average increasing rate of trans-membrane pressure increased, the stable filtration period was shortened, and the two stages (smooth stage and accelerating stage) of the trans-membrane pressure were more obvious. At the same time, the increasing rate of trans-membrane pressure at the smooth stage decreased and the rate at the accelerating stage increased with SVI, respectively. The observation by using scanning electronic microscopes showed the cake layer with loose structure and large thickness formed on the membrane surface due to the appearance of filamentous bacteria and high SVI in sludge. Influence of the sludge settleability on the trans-membrane pressure was related to the structure and thickness of the cake layer on the membrane.

关键词： Influence     bioreactor     activated     filamentous     lab-scale equipment    

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Biodegradation of trace pharmaceutical substances in wastewater by a membrane bioreactor

Longli BO, Taro URASE, Xiaochang WANG

《环境科学与工程前沿（英文）》 2009年 第3卷 第2期   页码 236-240 doi: 10.1007/s11783-009-0004-9

摘要： The biodegradation of selected pharmaceutical micropollutants, including two pharmaceuticals with argued biodegradation, was studied by a lab-scale membrane bioreactor. The reaction kinetics and affecting factors were also investigated in this paper. Clofibric acid (CA) with contradictive biodegradation reported was degraded almost completely at different hydraulic retention times (HRTs) after adaptation to microorganisms. The biodegradation of CA was disturbed at low pH operation, while the activity of microorganisms recovered again after pH adjustment to neutral condition. Ibuprofen (IBP) degraded under neutral and acidic conditions. Removals of IBP and CA were zero-order and first-order reactions under high and low initial concentrations, respectively. Carbamazepine and diclofenac were not degraded regardless of HRTs and pH.

关键词： pharmaceuticals     membrane bioreactor     activated sludge     reaction kinetics    

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Preliminary study of groundwater denitrification using a composite membrane bioreactor

Lihui ZHANG, Guomin CAO, Yulei FEI, Hong DING, Mei SHENG, Yongdi LIU

《环境科学与工程前沿（英文）》 2011年 第5卷 第4期   页码 604-609 doi: 10.1007/s11783-011-0274-x

摘要： A composite membrane bioreactor (CMBR) integrating the immobilized cell technique and the membrane separation technology was developed for groundwater denitrification. The CMBR had two well mixed compartments with one filled with the nitrate- containing influent and the other with a dilute ethanol solution; the compartments were separated by the composite membrane consisting of a microporous membrane facing the influent and an immobilized cell membrane facing the ethanol solution. Nitrate and ethanol molecules diffused from the respective compartments into the immobilized cell membrane where nitrate was reduced to gaseous nitrogen by the denitrifying bacteria present there with ethanol as the carbon source. The microporous membrane was attached to one side of the immobilized cell membrane for retention of the disaggregated bacteria. Relative to the single dose of external ethanol, the two-dose supplementation produced better treatment results as evidenced by the lower concentrations of and ethanol (as measured by total organic carbon) of the effluent. The batch treatment in CMBR removed most of the nitrate in the influent and attained a stable denitrification rate of 0.1 g·m ·h for most of the 96-h cycles during the 30-cycle study. The effluent was essentially free of ethanol and nitrite nitrogen.

关键词： groundwater     nitrate     denitrification     composite membrane bioreactor (CMBR)     immobilized cell membrane    

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Effects of a dynamic membrane formed with polyethylene glycol on the ultrafiltration of natural organic

Boksoon KWON, Noeon PARK, Jaeweon CHO,

《环境科学与工程前沿（英文）》 2010年 第4卷 第2期   页码 172-182 doi: 10.1007/s11783-010-0002-y

摘要： The formation of a dynamic membrane (DM) was investigated using polyethylene glycol (PEG) (molecular weight of 35000 g/mol, concentration of 1 g/L). Two natural organic matters (NOM), Dongbok Lake NOM (DLNOM) and Suwannee River NOM (SRNOM) were used in the ultrafiltration experiments along with PEG. To evaluate the effects of the DM with PEG on ultrafiltration, various transport experiments were conducted, and the analyses of the NOM in the membrane feed and permeate were performed using high performance size exclusion chromatography, and the pore size distribution ( PSD) and molecular weight cut off ( MWCO) were determined. The advantages of DM formed with PEG can be summarized as follows: (1) PEG interferes with NOM transmission through the ultrafiltration membrane pores by increasing the retention coefficient of NOM in UF membranes, and (2) low removal of NOM by the DM is affected by external factors, such as pressure increases during UF membrane filtration, which decreases the PSD and MWCO of UF membranes. However, a disadvantage of the DM with PEG was severe flux decline; thus, one must be mindful of both the positive and negative influences of the DM when optimizing the UF performance of the membrane.

关键词： dynamic membrane     natural organic matters     ultrafiltration membrane performance     effective PSD     effective molecular weight cutoff    

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标题 作者 时间 类型 操作

Development of combined coagulation-hydrolysis acidification-dynamic membrane bioreactor system for treatment

Xue Shen, Lei Lu, Baoyu Gao, Xing Xu, Qinyan Yue

期刊论文

Methanation and chemolitrophic nitrogen removal by an anaerobic membrane bioreactor coupled partial nitrification

期刊论文

Recent advances in membrane bioreactor technology for wastewater treatment in China

Xia HUANG, Kang XIAO, Yuexiao SHEN

期刊论文

Bisphenol A removal from synthetic municipal wastewater by a bioreactor coupled with either a forwardosmotic membrane or a microfiltration membrane unit

Hongtao ZHU, Wenna LI

期刊论文

Enhanced atrazine removal using membrane bioreactor bioaugmented with genetically engineered microorganism

LIU Chun, HUANG Xia

期刊论文

characteristics of wastewater treatment plants retrofitted from the conventional activated sludge process to the membranebioreactor process

期刊论文

Energy reduction of a submerged membrane bioreactor using a polytetrafluoroethylene (PTFE) hollow-fibermembrane

Taro Miyoshi, Thanh Phong Nguyen, Terumi Tsumuraya, Hiromu Tanaka, Toru Morita, Hiroki Itokawa, Toshikazu Hashimoto

期刊论文

Performance of bioferric-submerged membrane bioreactor for dyeing wastewater treatment

ZOU Haiyan, XI Danli

期刊论文

Membrane bioreactors for hospital wastewater treatment: recent advancements in membranes and processes

期刊论文

Engineering application of membrane bioreactor for wastewater treatment in China: Current state and future

Kang XIAO, Ying XU, Shuai LIANG, Ting LEI, Jianyu SUN, Xianghua WEN, Hongxun ZHANG, Chunsheng CHEN, Xia HUANG

期刊论文

Effects of hydraulic retention time on net present value and performance in a membrane bioreactor treating

Dawei Yu, Jianxing Wang, Libin Zheng, Qianwen Sui, Hui Zhong, Meixue Cheng, Yuansong Wei

期刊论文

Relationship between sludge settleability and membrane fouling in a membrane bioreactor

SUN Yujiao, WANG Yong, HUANG Xia

期刊论文

Biodegradation of trace pharmaceutical substances in wastewater by a membrane bioreactor

Longli BO, Taro URASE, Xiaochang WANG

期刊论文

Preliminary study of groundwater denitrification using a composite membrane bioreactor

Lihui ZHANG, Guomin CAO, Yulei FEI, Hong DING, Mei SHENG, Yongdi LIU

期刊论文

Effects of a dynamic membrane formed with polyethylene glycol on the ultrafiltration of natural organic

Boksoon KWON, Noeon PARK, Jaeweon CHO,

期刊论文